Tuesday, March 5, 2013

1303.0734 (E. Werner et al.)

Monomer distributions and intra-chain collisions of a polymer confined
to a channel
   [PDF]

E. Werner, F. Westerlund, J. O. Tegenfeldt, B. Mehlig
We study the conformations of a self-avoiding polymer confined to a channel by computing the cross-sectional distributions of the positions of its monomers. By means of Monte-Carlo simulations for a self-avoiding, freely-jointed chain we determine how the cross-sectional distribution for a given monomer depends on its location in the polymer, and how strongly this distribution is affected by self avoidance. To this end we analyze how the frequency of intra-chain collisions between monomers depends on their spatial position in the channel and on their location within the polymer. We show that most collisions occur between closely neighboring monomers. As a consequence the collision probability depends only weakly on the spatial position of the monomers. Our results explain why the effect of self-avoidance on the monomer distributions is weaker than predicted by mean-field theory. We discuss the relevance of our results for studies of DNA conformations in nanofluidic channels.
View original: http://arxiv.org/abs/1303.0734

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